Hey, guys, if this was the issue you were mentioning as Penguin's 1st Silver Age appearance, it is reprinted in Batman in the 60s in addition to the Arkham Penguin book. Each book in the Arkham series spotlights a single villain and there are several volumes.
http://www.mikesamazingworld.com/mikes/ ... micid=3682
I want to go at your analysis from the opposite, mirror direction. I first discovered Batman and his rogues watching reruns of the 1960s show in 1976, Penguin was the villain I found closest to his TV show image. That would have been in a David V. Reed two-parter in Batman 287-288. Admittedly, Reed's was the most light-hearted Batman of the Bronze Age. I also can see Englehart's Malay Penguin working as a TV show episode.
Next to Penguin, in the bronze age, I found Joker to be closest to his TV counterpart. While the Joker in the comics was certainly more murderous, in my two favorite bronze age issues, the Joker makes fish have his face and in the other one he straps his enemies to giant rocket candles on his birthday cake. The difference : in the comics everyone thinks these are crazy plots that don't make any sense. As Batman said, "The Joker's insane schemes make sense to him alone." On the TV show, every Gotham City citizen would have thought his plots made perfect sense.
The villain who was the most different was Riddler. I didn't like how much more calm and subdued he was in the comics after being wowed by Frank Gorshin's manic performance. The Riddler on Power Records Batman story was more Gorshin.
The "Four Birds of a Feather" Batman story from Batman 11 was later adapted into a Whitman Giant Comics to Color. I don't know why Whitman did a new adaptation and didn't just reprint actual comic book stories.
https://www.amazon.com/Batman-Robin-Bat ... B001KTQTJG